Burgess Meredith
Role: Dr. Diabolo (Framing Story)
Jack Palance
Role: Ronald Wyatt (segment 4 "The Man Who Collected Poe")
Beverly Adams
Role: Carla Hayes (segment 2 "Terror Over Hollywood")
Peter Cushing
Role: Lancelot Canning (segment 4 "The Man Who Collected Poe")
Maurice Denham
Role: Uncle Roger (segment 1 "Enoch")
Barbara Ewing
Role: Dorothy Endicott (segment 3 "Mr. Steinway")
Michael Bryant
Role: Colin Williams (segment 1 "Enoch")
John Standing
Role: Leo Winston (segment 3 "Mr. Steinway")
Robert Hutton
Role: Bruce Benton (segment 2 "Terror Over Hollywood")
John Phillips
Role: Eddie Storm (segment 2 "Terror Over Hollywood")
Michael Ripper
Role: Gordon Roberts (Framing Story)
Bernard Kay
Role: Dr. Heim (segment 2 "Terror Over Hollywood")
Catherine Finn
Role: Nurse Parker (segment 1 "Enoch")
Ursula Howells
Role: Miss Maxine Chambers (segment 3 "Mr. Steinway")
David Bauer
Role: Mike Charles (segment 2 "Terror Over Hollywood")
Niall MacGinnis
Role: Dr. Silversmith (segment 1 "Enoch")
Hedger Wallace
Role: Edgar Allan Poe(segment "4 "The Man Who Collected Poe"")
